A laser-based technique for measuring instantaneous three-dimensional species concn. distributions in turbulent flows is presented. The laser beam from a single laser is formed into two crossed light sheets that illuminate the area of interest. The laser-induced fluorescence (LIF) signal emitted from excited species within both planes is detected with a single camera via a mirror arrangement. Image processing enables the reconstruction of the three-dimensional data set in close proximity to the cutting line of the two light sheets. Three-dimensional intensity gradients are computed and compared to the two-dimensional projections obtained from the two directly obsd. planes. Vol. visualization by digital image processing gives unique insight into the three-dimensional structures within the turbulent processes. The authors apply this technique to measurements of toluene-LIF in a turbulent, nonreactive mixing process of toluene and air and to hydroxyl (OH) LIF in a turbulent methane-air flame upon excitation at 248 nm with a tunable KrF excimer laser.