Dreher, Pascal; Janoschka, David; Neuhaus, Alexander; Frank, Bettina; Giessen, Harald; Horn-von Hoegen, Michael; Meyer zu Heringdorf, Frank:
Quantitative determination of the electric field strength in a plasmon focus from ponderomotive energy shifts
In: Nanophotonics, Vol. 11 (2022), No. 16, pp. 3687 - 3694
2022article/chapter in journalOA Gold
Physics (incl. Astronomy)Faculty of Physics » Experimental PhysicsScientific institutes » Center for Nanointegration Duisburg-Essen (CENIDE)
Related: 1 publication(s)
Title in English:
Quantitative determination of the electric field strength in a plasmon focus from ponderomotive energy shifts
Author:
Dreher, PascalUDE
LSF ID
60601
ORCID
0000-0001-8975-1983ORCID iD
Other
connected with university
;
Janoschka, DavidUDE
LSF ID
57798
ORCID
0000-0002-4311-330XORCID iD
Other
connected with university
;
Neuhaus, Alexander;Frank, Bettina;Giessen, Harald;Horn-von Hoegen, MichaelUDE
GND
1201039908
LSF ID
10366
ORCID
0000-0003-0324-3457ORCID iD
Other
connected with university
;
Meyer zu Heringdorf, FrankUDE
LSF ID
48700
ORCID
0000-0002-5878-2012ORCID iD
Other
connected with university
corresponding author
Year of publication:
2022
Open Access?:
OA Gold
DuEPublico 2 ID
Web of Science ID
Scopus ID
Note:
OA Förderung 2022
Language of text:
English
Keyword, Topic:
photoelectron spectroscopy; photoemission microscopy; ponderomotive energy; surface plasmon polariton

Abstract in English:

Spectroscopic photoemission microscopy is used to detect and quantify a ponderomotive shift in the energy of electrons that are emitted from a surface plasmon polariton focus. The focus is formed on an atomically flat Au(111) surface by an Archimedean spiral and is spatiotemporally separated from the circularly polarized light pulse used to excite the spiral. A spectroscopic analysis of electrons emitted from the focus exhibits a peaked above-threshold electron emission spectrum. From the shift of the peaks as function of laser power the field strength of the surface plasmon polariton was quantitatively determined without free parameters. Estimations of the Keldysh parameter γ = 4.4 and the adiabaticity parameter δ = 4700 indicate that electron emission occurs in a regime of multiplasmon absorption and nonlocalized surface plasmon fields.