Le Guyader, Loïc; Eschenlohr, Andrea; Beye, Martin; Schlotter, William; Döring, Florian; Carinan, Cammille; Hickin, David; Agarwal, Naman; Boeglin, Christine; Bovensiepen, Uwe; Buck, Jens; Carley, Robert; Castoldi, Andrea; D'Elia, Alessandro; Delitz, Jan Torben; Delitz, Jan-Torben et al:
Photon-shot-noise-limited transient absorption soft X-ray spectroscopy at the European XFEL
In: Journal of Synchrotron Radiation, Vol. 30 (2023), No. 2, pp. 284 - 300
2023article/chapter in journalOA Gold
Physics (incl. Astronomy)Faculty of PhysicsScientific institutes » Center for Nanointegration Duisburg-Essen (CENIDE)
Related: 1 publication(s)
Title in English:
Photon-shot-noise-limited transient absorption soft X-ray spectroscopy at the European XFEL
Author:
Le Guyader, Loïc
Other
corresponding author
;
Eschenlohr, AndreaUDE
LSF ID
55024
ORCID
0000-0002-0814-3511ORCID iD
Other
connected with university
;
Beye, Martin
;
Schlotter, William
;
Döring, Florian
;
Carinan, Cammille
;
Hickin, David
;
Agarwal, Naman
;
Boeglin, Christine
;
Bovensiepen, UweUDE
GND
122280083
LSF ID
51228
ORCID
0000-0002-1506-4491ORCID iD
Other
connected with university
;
Buck, Jens
;
Carley, Robert
;
Castoldi, Andrea
;
D'Elia, Alessandro
;
Delitz, Jan Torben
;
Ehsan, Wajid
;
Engel, Robin
;
Erdinger, Florian
;
Fangohr, Hans
;
Fischer, Peter
;
Fiorini, Carlo
;
Föhlisch, Alexander
;
Gelisio, Luca
;
Gensch, Michael
;
Gerasimova, Natalia
;
Gort, Rafael
;
Hansen, Karsten
;
Hauf, Steffen
;
Izquierdo, Manuel
;
Jal, Emmanuelle
;
Kamil, Ebad
;
Karabekyan, Suren
;
Kluyver, Thomas
;
Laarmann, Tim
;
Lojewski, Tobias
;
Lomidze, David
;
Maffessanti, Stefano
;
Mamyrbayev, Talgat
;
Marcelli, Augusto
;
Mercadier, Laurent
;
Mercurio, Giuseppe
;
Miedema, Piter S.
;
Ollefs, KatharinaUDE
LSF ID
50617
ORCID
0000-0002-2301-4670ORCID iD
Other
connected with university
;
Rossnagel, Kai
;
Rösner, Benedikt
;
Rothenbach, NicoUDE
GND
1220951854
LSF ID
58445
ORCID
0000-0002-2592-5857ORCID iD
Other
connected with university
;
Samartsev, Andrey
;
Schlappa, Justine
;
Setoodehnia, Kiana
;
Sorin Chiuzbaian, Gheorghe
;
Spieker, LeaUDE
LSF ID
61938
ORCID
0000-0002-3944-2696ORCID iD
Other
connected with university
;
Stamm, Christian
;
Stellato, Francesco
;
Techert, Simone
;
Teichmann, Martin
;
Turcato, Monica
;
Van Kuiken, Benjamin
;
Wende, HeikoUDE
GND
12115226X
LSF ID
47290
ORCID
0000-0001-8395-3541ORCID iD
Other
connected with university
;
Yaroslavtsev, Alexander
;
Zhu, Jun
;
Molodtsov, Serguei
;
David, Christian
;
Porro, Matteo
;
Scherz, Andreas
;
Delitz, Jan-Torben
Year of publication:
2023
Open Access?:
OA Gold
PubMed ID
Scopus ID
Note:
CA extern
Language of text:
English
Keyword, Topic:
European XFEL ; transient absorption soft X-ray spectroscopy

Abstract in English:

Femtosecond transient soft X-ray absorption spectroscopy (XAS) is a very promising technique that can be employed at X-ray free-electron lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here, a dedicated setup for soft X-rays available at the Spectroscopy and Coherent Scattering (SCS) instrument at the European X-ray Free-Electron Laser (European XFEL) is presented. It consists of a beam-splitting off-axis zone plate (BOZ) used in transmission to create three copies of the incoming beam, which are used to measure the transmitted intensity through the excited and unexcited sample, as well as to monitor the incoming intensity. Since these three intensity signals are detected shot by shot and simultaneously, this setup allows normalized shot-by-shot analysis of the transmission. For photon detection, an imaging detector capable of recording up to 800 images at 4.5 MHz frame rate during the FEL burst is employed, and allows a photon-shot-noise-limited sensitivity to be approached. The setup and its capabilities are reviewed as well as the online and offline analysis tools provided to users.