Dreher, Pascal; Janoschka, David; Frank, Bettina; Giessen, Harald; Meyer zu Heringdorf, Frank-J.:
Focused surface plasmon polaritons coherently couple to electronic states in above-threshold electron emission
In: Communications Physics, Jg. 6 (2023), Heft 1, Artikel 15
2023Artikel/Aufsatz in ZeitschriftOA Gold
Physik (inkl. Astronomie)Fakultät für PhysikForschungszentren » Center for Nanointegration Duisburg-Essen (CENIDE)
Damit verbunden: 1 Publikation(en)
Titel in Englisch:
Focused surface plasmon polaritons coherently couple to electronic states in above-threshold electron emission
Autor*in:
Dreher, PascalUDE
LSF ID
60601
ORCID
0000-0001-8975-1983ORCID iD
Sonstiges
der Hochschule zugeordnete*r Autor*in
korrespondierende*r Autor*in
;
Janoschka, DavidUDE
LSF ID
57798
ORCID
0000-0002-4311-330XORCID iD
Sonstiges
der Hochschule zugeordnete*r Autor*in
;
Frank, Bettina
;
Giessen, Harald
;
Meyer zu Heringdorf, Frank-J.UDE
LSF ID
48700
Sonstiges
der Hochschule zugeordnete*r Autor*in
Erscheinungsjahr:
2023
Open Access?:
OA Gold
DuEPublico 2 ID
Scopus ID
Notiz:
OA Förderung 2023
Sprache des Textes:
Englisch
Ressourcentyp:
Text

Abstract in Englisch:

When an intense light field strongly interacts with the band structure of a solid, the formation of hybrid light-matter quantum states becomes possible. Examples of such Floquet-Bloch states have been reported, but engineering of the band structure using Floquet states can suffer from dissipation and decoherence. Sustaining the necessary quantum coherence of the light-matter interactions requires robust electronic states in combination with strong fields of suitable polarization and frequency. Here, we explore the quantum coherent coupling of nano-focused surface plasmon polaritons (SPP) to distinct electronic states in the band structure of a solid. We observe above-threshold electron emission from the Au(111) Shockley surface state by the absorption of up to seven SPP quanta. Using time-resolved photoelectron spectroscopy the coherence of the interaction of the SPPs with the surface state during electron emission is investigated and the process is shown to be similar to light-driven above threshold electron emission. Ultimately, our work could render SPP-based Floquet engineering in nano-optical systems feasible.